Femtosecond signatures of optically induced magnons before ultrafast demagnetization

Optically induced demagnetization of 3d metallic ferromagnets proceeds as fast as ~100 fs and is a crucial prerequisite for spintronic applications, such as ultrafast magnetization switching and spin transport. On the 100 fs time scale, the magnetization dynamics is widely understood in the context of temperature models considering energy transfers between conduction electrons, magnons and crystal lattice. However, on even faster time scales, the flow of both angular momentum and energy between these subsystems has so far not been studied. Here, we measure ultrafast demagnetization by ultrabroadband THz-emission spectroscopy. We find that the rate of change of the magnetization does not rise instantaneously, but on a time scale shorter than 10 fs. In the framework of a general model of the three interacting subsystems, this rise is a signature that a transfer of angular momentum from magnons to conduction electrons proceeds in less than 10 fs, before substantial demagnetization has happened. We further conclude that most of the spin dissipated by the crystal lattice is transferred via magnon-lattice rather than electron-lattice interaction. Our results show that the limiting speed of magnetization dynamics is not quenching of magnetic order and harnessing the earliest magnon dynamics could be a new route towards even faster spintronics.