Spin light-emitting devices in a 2D magnet

Emerging two-dimensional (2D) magnetic semiconductors represent transformative platforms to explore magneto-optics and opto-spintronic applications. Though 2D opto-spintronics has attracted tremendous research efforts in spin-dependent photodetectors and non-volatile memory components, the realization of one core application -spin-modulated light-emitting device (spin-LED)- remains elusive so far. Here we successfully realize prototype spin-LED integrated with a 2D semiconducting magnet CrSBr, demonstrating considerable electroluminescence (EL) down to bilayers. Intriguingly, the EL of the spin-LED is discovered to be directly manipulated by spin-flip and spin-canting transitions. Notably, spin-flip transitions enable unprecedented hysteretic behaviors of EL characteristics, while spin-canting transitions induce EL continuous modulation with robust anisotropy. This versatile manipulation is originated from the synergy of magnetic-order mediated excitonic transitions and spintronic transport. The prototype demonstration of spin-LED establishes an indispensable scheme of opto-spintronic devices leveraging 2D spin transitions and strong excitonic effects, presenting a critical step towards integrated 2D opto-spintronics.