Controlling the morphology transition on MOVPE-grown (100) β-Ga2O3 film between step-flow growth and step-bunching: A machine learning-assisted approach
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The step-bunching instability in (100) β-Ga₂O₃ films grown via metalorganic vapor phase epitaxy (MOVPE) was investigated using a machine learning approach based on Random Forest (RF). The study reveals the interplay of Ga supersaturation (O 2 /Ga) and impurity effects as coexisting mechanisms driving the morphological transition (from step-flow growth to step-bunching). The developed machine-learning framework accurately classifies growth morphology and offers valuable insights by correlating theoretical principles with experimental parameters. Critical growth parameters influencing the film morphology were identified. The corresponding strategy, high Ga supersaturation, is proposed to mitigate the step-bunching formation and maintain the desired step-flow growth mode. Despite the challenges posed by small datasets, the RF model demonstrates robust classification performance, establishing machine learning as a powerful tool for experimental science.
