Investigating the Magnetocaloric Effect of GdGaAl Alloys Using Mean-Field Theory

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Abstract

In this paper, we investigated the magnetocaloric properties and magnetic parameters of GdGa 1 − x Al x (0≤𝑥≤0.5) alloys using mean-field theory. The magnetization, exchange field, and magnetic entropy change are examined to understand how partial substitution of Ga with Al affects these properties. The magnetocaloric effect (MCE) shows promising results, with maximum entropy changes of 3.40, 2.94, and 4.20 J·kg⁻¹·K⁻¹ under 0–2 T change magnetic field for x=0, 0.3, and 0.5, respectively. The temperature-averaged entropy change (𝑇𝐸𝐶) values remain stable across a wide temperature range, making these materials suitable for refrigeration applications. The highest 𝑇𝐸𝐶 of 9.50 J·kg⁻¹·K⁻¹ is observed for the x = 0.5 alloy, indicating enhanced magnetocaloric performance with higher Al content.

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