Quantifying the Impact of Atmospheric Aerosols on Clear-Sky and All-Sky Solar Irradiance Components in a Tropical Coastal Urban Environment: A Case Study of Penang, Malaysia (2014–2018)

Atmospheric aerosols strongly regulate surface solar irradiance in tropical coastal environments through scattering and absorption. This study examines aerosol–irradiance interactions over Penang, Malaysia, using Aerosol Robotic Network (AERONET) observations of aerosol optical depth (AOD), single scattering albedo (SSA), and extinction Ångström exponent (AE); NASA’s Prediction of Worldwide Energy Resource (POWER) irradiance data; and MERRA-2 reanalysis for aerosol compositional context. Bottom-of-atmosphere radiative forcing efficiency (BOA RFE) was quantified for global, direct and diffuse irradiance (GHI, DNI and DHI) under clear and all-sky conditions during 2014–2018. Results show persistent aerosol-induced attenuation of surface radiation, with GHI and DNI RFE predominantly negative, while DHI RFE remains consistently positive, indicating redistribution of solar energy from direct to diffuse components. Time resolved analysis reveals daily GHI RFE typically ranging from approximately −0.5 to −3.5 W m⁻² per unit AOD, with episodic excursions below −4 W m⁻² per AOD during high-aerosol events, whereas DNI RFE frequently reaches values below −0.8 W m⁻² per AOD, confirming its greater sensitivity to aerosol extinction. In contrast, DHI RFE commonly exceeds +5 W m⁻² per AOD and intermittently surpasses +10 W m⁻² per AOD, reflecting enhanced scattering and multiple-scattering effects. AOD-stratified analysis demonstrates a nonlinear weakening of forcing efficiency with increasing aerosol burden, with mean GHI RFE decreasing from approximately −1.6 to −0.4 W m⁻² per AOD between low- and high-AOD regimes, accompanied by corresponding reductions in DNI (−0.35 to −0.1 W m⁻² per AOD) and DHI (+3.3 to +0.8 W m⁻² per AOD). Overall, aerosol loading is identified as the dominant control on BOA radiative forcing efficiency in this tropical coastal environment, while SSA and AE act as secondary modulators.